{"created":"2023-06-20T15:28:43.968855+00:00","id":8233,"links":{},"metadata":{"_buckets":{"deposit":"68d2d264-eef6-4e10-aebf-8a4bd68bd504"},"_deposit":{"created_by":12,"id":"8233","owners":[12],"pid":{"revision_id":0,"type":"depid","value":"8233"},"status":"published"},"_oai":{"id":"oai:ouj.repo.nii.ac.jp:00008233","sets":["389:535"]},"author_link":["10563","10562"],"item_10001_biblio_info_7":{"attribute_name":"書誌情報","attribute_value_mlt":[{"bibliographicIssueDates":{"bibliographicIssueDate":"2009-07-28","bibliographicIssueDateType":"Issued"},"bibliographicPageStart":"035430","bibliographicVolumeNumber":"80","bibliographic_titles":[{"bibliographic_title":"Physical Review B"}]}]},"item_10001_description_5":{"attribute_name":"抄録","attribute_value_mlt":[{"subitem_description":"We present a nuclear wave-packet simulation of photoinduced coherent adsorbate dynamics on a metal surface with quasi-diabatic potential energy curves obtained from our recently developed open-boundary cluster model approach. Photoexcitation to the resonant adsorbate state and the subsequent ultrafast decay to the electronically excited substrate states were found to cause a coherent vibration of the adsorbate on the metal surface. This process competes with a Raman scattering process, which is generally believed to explain the coherent adsorbate vibration. These two mechanisms induce vibrations with a common frequency, and therefore cannot be distinguished from each other in a frequency-domain experiment. However, they can be distinguished by determining the initial vibrational phase through a time domain experiment such as ultrafast pump-probe spectroscopy. We further demonstrate that for near-resonant excitation the oscillation amplitude induced by our proposed mechanism largely exceeds the amplitude due to the Raman mechanism.","subitem_description_type":"Abstract"}]},"item_10001_relation_14":{"attribute_name":"DOI","attribute_value_mlt":[{"subitem_relation_type":"isIdenticalTo","subitem_relation_type_id":{"subitem_relation_type_id_text":"10.1103/PhysRevB.80.035430","subitem_relation_type_select":"DOI"}}]},"item_10001_rights_15":{"attribute_name":"権利","attribute_value_mlt":[{"subitem_rights":"© 2009 The American Physical Society"}]},"item_10001_source_id_9":{"attribute_name":"ISSN","attribute_value_mlt":[{"subitem_source_identifier":"1098-0121","subitem_source_identifier_type":"ISSN"}]},"item_10001_version_type_20":{"attribute_name":"著者版フラグ","attribute_value_mlt":[{"subitem_version_resource":"http://purl.org/coar/version/c_970fb48d4fbd8a85","subitem_version_type":"VoR"}]},"item_creator":{"attribute_name":"著者","attribute_type":"creator","attribute_value_mlt":[{"creatorNames":[{"creatorName":"YASUIKE, Tomokazu"}],"nameIdentifiers":[{"nameIdentifier":"10562","nameIdentifierScheme":"WEKO"}]},{"creatorNames":[{"creatorName":"NOBUSADA, Katsuyuki"}],"nameIdentifiers":[{"nameIdentifier":"10563","nameIdentifierScheme":"WEKO"}]}]},"item_files":{"attribute_name":"ファイル情報","attribute_type":"file","attribute_value_mlt":[{"accessrole":"open_date","date":[{"dateType":"Available","dateValue":"2014-10-31"}],"displaytype":"detail","filename":"2009-PRB80.pdf","filesize":[{"value":"367.7 kB"}],"format":"application/pdf","licensetype":"license_note","mimetype":"application/pdf","url":{"label":"Photoinduced coherent adsorbate dynamics on a metal surface","url":"https://ouj.repo.nii.ac.jp/record/8233/files/2009-PRB80.pdf"},"version_id":"ffb95193-68ba-40b4-ad46-e291605e6d9c"}]},"item_language":{"attribute_name":"言語","attribute_value_mlt":[{"subitem_language":"eng"}]},"item_resource_type":{"attribute_name":"資源タイプ","attribute_value_mlt":[{"resourcetype":"journal article","resourceuri":"http://purl.org/coar/resource_type/c_6501"}]},"item_title":"Photoinduced coherent adsorbate dynamics on a metal surface: Nuclear wave-packet simulation with quasi-diabatic potential energy curves using an open-boundary cluster model approach","item_titles":{"attribute_name":"タイトル","attribute_value_mlt":[{"subitem_title":"Photoinduced coherent adsorbate dynamics on a metal surface: Nuclear wave-packet simulation with quasi-diabatic potential energy curves using an open-boundary cluster model approach"},{"subitem_title":"Photoinduced coherent adsorbate dynamics on a metal surface: Nuclear wave-packet simulation with quasi-diabatic potential energy curves using an open-boundary cluster model approach","subitem_title_language":"en"}]},"item_type_id":"10001","owner":"12","path":["535"],"pubdate":{"attribute_name":"公開日","attribute_value":"2014-10-31"},"publish_date":"2014-10-31","publish_status":"0","recid":"8233","relation_version_is_last":true,"title":["Photoinduced coherent adsorbate dynamics on a metal surface: Nuclear wave-packet simulation with quasi-diabatic potential energy curves using an open-boundary cluster model approach"],"weko_creator_id":"12","weko_shared_id":12},"updated":"2023-06-20T16:11:28.504434+00:00"}